Zakynthos has many many small villages all around. It certainly worth while visiting a few to grasp the rhythm of local rural life.
If you want to feel a little bohemian you should pay a visit to the Marathia plates.
The plateau of Iperagathos Monastery with a plain that stretches continuously. Suited to everyone
Iperagathos MTB trail
Amazing ride through a plateau with mixed forest and agricultural landscape. Suitable for MTB enthusiasts